Thermomechanical action of ultrashort laser pulses on metallic nanostructures

Содержание

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Damping oscillations: M. Perner, S. Gresillon, J. März, G. von Plessen,


Damping oscillations:

M. Perner, S. Gresillon, J. März, G. von Plessen, J. Feldmann // Phys. Rev. Lett.

2000. V.85. P.792.

pump – probe spectroscopy

Excitation of acoustic vibrations in spherical metallic nanoparticles

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Laser-induced explosion of gold nanoparticles: potential role for nanophotothermolysis of cancer


Laser-induced explosion of gold nanoparticles: potential role for nanophotothermolysis of

cancer

R. Letfullin, Ch. Joenathan, Th. George, V. Zharov // Nanomedicine, 2006, V.1. P.473.

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Cavitation phenomena around nanoparticles Gold nanoparticle targeted photoacoustic cavitation for potential


Cavitation phenomena around nanoparticles

Gold nanoparticle targeted photoacoustic cavitation for

potential deep tissue imaging and therapy / Hengyi Ju, Ronald A. Roy, and Todd W. Murray // BIOMEDICAL OPTICS EXPRESS 2013 / Vol. 4, No. 1 P. 66

(a) Acoustic signals from a photoacoustic cavitation event and a non-event around gold nanospheres (2.2 × 108 nanoparticles/ml) at a peak negative HIFU pressure of 1.5 MPa and a laser fluence of 4.8 mJ/cm2. (b) Cavitation probability as a function of laser fluence around gold nanospheres (2.2 × 108 nanoparticles/ml) at peak negative pressures of 1.5, 2.0, 2.5 and 3.0 MPa.

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Excitation of acoustic vibrations in nonspherical metallic nanoparticles Damping of acoustic


Excitation of acoustic vibrations in nonspherical metallic nanoparticles

Damping of acoustic

vibrations in gold
nanoparticles. Matthew Pelton, John E. Sader, Julien Burgin, Mingzhao Liu, Philippe Guyot-Sionnest and David Gosztola // NATURE NANOTECHNOLOGY VOL 4 2009 P.492

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Photothermal Cancer Therapy and Imaging Based on Gold Nanorods WON IL


Photothermal Cancer Therapy and Imaging Based on Gold Nanorods
WON IL

CHOI, ABHISHEK SAHU, YOUNG HA KIM, and GIYOONG TAE // Annals of Biomedical Engineering (2011)
DOI: 10.1007/s10439-011-0388-0

Excitation of acoustic vibrations in nonspherical metallic nanoparticles

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Excitation of shock waves under absorption of laser radiation in metallic


Excitation of shock waves under absorption
of laser radiation in

metallic films

Ultrashort strain solitons in sapphire and ruby / Otto Muskens et.al.

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Hypersonic Modulation of Light in Three-Dimensional Photonic and Phononic Band-Gap Materials


Hypersonic Modulation of Light in Three-Dimensional Photonic and Phononic Band-Gap

Materials

A. V. Akimov, Y. Tanaka, A. B. Pevtsov, S. F. Kaplan, V. G. Golubev, S. Tamura, D. R. Yakovlev, and M. Bayer // Phys. Rev. Lett. 101, 033902

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Main stages of thermooptical excitation of acoustic pulse: -absorption of laser


Main stages of thermooptical excitation of acoustic pulse:
-absorption of laser

pulse energy;
local heating;
local pressure increasing;
expansion due to gradient of pressure;
formation of acoustic pulse;
relaxation process.

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The Lagrange equations for the one-dimensional motion of a continuous medium

The Lagrange equations for the one-dimensional motion of a continuous medium

have the following form [1]:

– continuity equation

– motion equation

– equation of the changing of Euler coordinate R

– Mie–Grünheisen state equation

P (r,t),
u (r,t),
(r,t)
T (r,t)

α=1 – plane
α=2 – cylindrical
α=3 – spherical geometry

– heat transfer equation

[1] O.G. Romanov, G.I. Zheltov, G.S. Romanov. Numerical modeling of thermomechanical processes in absorption of laser radiation in spatially inhomogeneous media // Journal of Engineering Physics and Thermophysics, 2011. Vol. 84, No. 4, P.772-780.

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Peculiarities of the problem: - size of metallic structures (10-100 nm);


Peculiarities of the problem:
- size of metallic structures (10-100 nm);
-

pulse duration (100 fs).

Scheme of radiation–medium interaction in the plane (a), cylindrical (b), and spherical (c) geometries.

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- particle size (10-100nm); - pulse duration (100fs); Fast dynamics in small area 12


- particle size (10-100nm);
- pulse duration (100fs);

Fast dynamics in small

area

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heat source function electron-phonon relaxation The heating of metals with ultra


heat source function

electron-phonon relaxation

The heating of metals with ultra short

laser pulses is described by a two-temperature model for an electron gas and an ionic lattice:

S.I.Anisimov, Ya.A. Imas, G.S. Romanov, and Yu.V. Khodyko.
The Effect of High Power Radiation onto Metals, 1970 (in Russian).

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Mie–Grünheisen state equation for metallic nanoparticle: Mie–Grünheisen state equation for environment: 14

Mie–Grünheisen state equation for metallic nanoparticle:

Mie–Grünheisen state equation for environment:

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Lagrange equations [2]: Artificial viscosity [2] R.D. Richtmayer, and K.W. Morton,

Lagrange equations [2]:

Artificial viscosity

[2] R.D. Richtmayer, and K.W. Morton, Difference Methods

for Initial Value Problems, 1967.

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Heat transfer equation [3]: [3] V.K. Saul’ev, Parabolic Equations Integration by

Heat transfer equation [3]:

[3] V.K. Saul’ev, Parabolic Equations Integration by Grid

Method, 1960
(in Russian).

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Plane geometry α=1 Space distributions of temperature (а), velocity (b) and

Plane geometry
α=1

Space distributions of temperature (а), velocity (b) and pressure

(c, d) in different time moments.
1 – 100 fs, 2 – 500 fs, 3 – 1 ps, 4 – 2 ps, 5 – 3 ps, 6 – 4 ps, 7 – 5 ps

a

b

c

d

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Cylindrical geometry α=2 a Space distributions of temperature (а), velocity (b)

Cylindrical geometry
α=2

a

Space distributions of temperature (а), velocity (b) and pressure (c, d)

in different time moments.
1 – 100 fs, 2 – 500 fs, 3 – 1 ps, 4 – 2 ps, 5 – 3 ps, 6 – 4 ps, 7 – 5 ps

б

c

d

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Time dependences of temperature in the centre of gold nanoparticle Spherical

Time dependences of temperature in the centre of gold nanoparticle

Spherical geometry:

gold nanoparticle in water

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Сферическая геометрия α=3 Space distributions of temperature (а), velocity (b) and

Сферическая геометрия
α=3

Space distributions of temperature (а), velocity (b) and pressure

(c, d) in different time moments.
1 – 100 fs, 2 – 500 fs, 3 – 1 ps, 4 – 2 ps, 5 – 3 ps, 6 – 4 ps, 7 – 5 ps

a

b

c

d

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Oscillations of nanoparticle Spherical geometry: gold nanoparticle in water 21

Oscillations of nanoparticle

Spherical geometry: gold nanoparticle in water

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Pressure oscillations outside the particle (r =1nm from surface). Spherical geometry:

Pressure oscillations outside the particle (r =1nm from surface).

Spherical geometry: gold

nanoparticle in water

tp=10-13s, I0=1010 W/cm2

tp=10-11s, I0=108 W/cm2

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Gold nanoparticles in water (excitation by series of short pulses) Resonance

Gold nanoparticles in water
(excitation by series of short pulses)

Resonance enhancement

of the oscillation amplitude

Oscillations of nanoparticle (а) and temperature in the centre of particle (b).
1 – single pulse; 2, 3 – series of pulses. R0=10 nm; τp=10-13 s; I0=1010 W/cm2;
ν = 160GHz (2), 320GHz (3).

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Pressure oscillations outside the particle (r =1nm from surface). 1 -

Pressure oscillations outside the particle (r =1nm from surface). 1 - single

pulse;
2 – series of pulses, ν = 160GHz

Gold nanoparticles in water
(excitation by series of short pulses)

Resonance enhancement of the oscillation amplitude

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